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Abstract. Accurate boundary layer temperature and humidity profiles are crucial for successful forecasting of fog, and accurate retrievals of liquid water path are important for understanding the climatological significance of fog. Passive ground-based remote sensing systems such as microwave radiometers (MWRs) and infrared spectrometers like the Atmospheric Emitted Radiance Interferometer (AERI), which measures spectrally resolved infrared radiation (3.3 to 19.2 µm), can retrieve both thermodynamic profiles and liquid water path. Both instruments are capable of long-term unattended operation and have the potential to support operational forecasting. Here we compare physical retrievals of boundary layer thermodynamic profiles and liquid water path during 12 cases of thin (LWP<40 g m−2) supercooled radiation fog from an MWR and an AERI collocated in central Greenland. We compare both sets of retrievals to in-situ measurements from radiosondes and surface-based temperature and humidity sensors. The retrievals based on AERI observations accurately capture shallow surface-based temperature inversions (0–10 m a.g.l.) with lapse rates of up to −1.2 ∘C m−1, whereas the strength of the surface-based temperature inversions retrieved from MWR observations alone are uncorrelated with in-situ measurements, highlighting the importance of constraining MWR thermodynamic profile retrievals with accurate surface meteorological data. The retrievals based on AERI observations detect fog onset (defined by a threshold in liquid water path) earlier than those based on MWR observations by 25 to 185 min. We propose that, due to the high sensitivity of the AERI instrument to near-surface temperature and small changes in liquid water path, the AERI (or an equivalent infrared spectrometer) could be a useful instrument for improving fog monitoring and nowcasting, particularly for cases of thin radiation fog under otherwise clear skies, which can have important radiative impacts at the surface. 

Supercooled fogs can have an important radiative impact at the surface of the Greenland Ice Sheet, but they are difficult to detect and our understanding of the factors that control their lifetime and radiative properties is limited by a lack of observations. This study demonstrates that spectrally resolved measurements of downwelling longwave radiation can be used to generate retrievals of fog microphysical properties (phase and particle effective radius) when the fog visible optical depth is greater than ∼0.25. For 12 cases of fog under otherwise clear skies between June and September 2019 at Summit Station in central Greenland, nine cases were mixed‐phase. The mean ice particle (optically‐equivalent sphere) effective radius was 24.0 ± 7.8 µm, and the mean liquid droplet effective radius was 14.0 ± 2.7 µm. These results, combined with measurements of aerosol particle number concentrations, provide evidence supporting the hypotheses that (a) low surface aerosol particle number concentrations can limit fog liquid water path, (b) fog can act to increase near‐surface aerosol particle number concentrations through enhanced mixing, and (c) multiple fog events in quiescent periods gradually deplete near‐surface aerosol particle number concentrations.

 

Abstract. This study presents the first full annual cycle (2019–2020) of ambient surface aerosol particle number concentration measurements (condensationnuclei > 20 nm, N20) collected at Summit Station (Summit), in the centre of the Greenland Ice Sheet (72.58∘ N, −38.45∘ E; 3250 ma.s.l.). The mean surface concentration in 2019 was 129 cm−3, with the 6 h mean ranging between 1 and 1441 cm−3. The highest monthly mean concentrations occurred during the late spring and summer, with the minimum concentrations occurring in February (mean: 18 cm−3). High-N20 events are linked to anomalous anticyclonic circulation over Greenland and the descent of free-tropospheric aerosol down to the surface, whereas low-N20 events are linked to anomalous cyclonic circulation over south-east Greenland that drives upslope flow and enhances precipitation en route to Summit. Fog strongly affects particle number concentrations, on average reducing N20 by 20 % during the first 3 h of fog formation. Extremely-low-N20 events (< 10 cm−3) occur in all seasons, and we suggest that fog, and potentially cloud formation, can be limited by low aerosol particle concentrations over central Greenland. 

The tropical Andes of southern Peru and northern Bolivia have several major mountain summits suitable for ice core paleoclimatic investigations. However, incomplete understanding of the controls on the isotopic ( δD, δ¹⁸O) composition of precipitation and a paucity of field observations in this region continue to limit ice-core-based paleoclimate reconstructions. This study examines four years of daily observations of δD and δ¹⁸O in precipitation from a citizen scientist network on the northeastern margin of the Altiplano, to identify controls on the subseasonal spatiotemporal variability in δ¹⁸O during the wet season (November–April). These data provide new insights into modern δ¹⁸O variability at high spatial and temporal scales. We identify a regionally coherent subseasonal signal in precipitation δ¹⁸O featuring alternating periods of high and low δ¹⁸O of 9–27-day duration. This signal reflects variability in precipitation delivery driven by synoptic conditions and closely relates to variations in the strength of the South American low-level jet and moisture availability over the study area. The annual layer of snowpack on the Quelccaya Ice Cap observed in the subsequent dry season retains this subseasonal signal, allowing the development of a snow-pit age model based on precipitation δ¹⁸O measurements, and demonstrating how synoptic variability is transmitted from the atmosphere to mountaintop snowpacks along the Altiplano’s eastern margin. This result improves our understanding of the hydrometeorological processes governing δ¹⁸O and δD in tropical Andean precipitation and has implications for improving paleoclimate reconstructions from tropical Andean ice cores and other paleoclimate records.